工业水处理 ›› 2020, Vol. 40 ›› Issue (3): 93-97. doi: 10.11894/iwt.2019-0232

• 试验研究 • 上一篇    下一篇

镨掺杂氧化锌声光催化降解苯酚的研究

袁玲玲(),罗正维,江晖,吴浪,耿文华*()   

  1. 南京工业大学生物与制药工程学院, 江苏南京 211816
  • 收稿日期:2019-12-30 出版日期:2020-03-20 发布日期:2020-03-20
  • 通讯作者: 耿文华 E-mail:470499890@qq.com;gengwenhua@njtech.edu.cn
  • 作者简介:袁玲玲(1993—),硕士。电话:18402568104, E-mail:470499890@qq.com

Sonophotocatalytic degradation of phenol in the presence of Pr-doped ZnO catalyst

Linlin Yuan(),Zhengwei Luo,Hui Jiang,Lang Wu,Wenhua Geng*()   

  1. College of Biotechnology and Pharmaceutical Engineering, Nanjing Tech University, Nanjing 211816, China
  • Received:2019-12-30 Online:2020-03-20 Published:2020-03-20
  • Contact: Wenhua Geng E-mail:470499890@qq.com;gengwenhua@njtech.edu.cn

摘要:

共沉淀法合成了镨掺杂的氧化锌(Pr-ZnO),并利用X射线衍射、扫描电子显微镜和紫外可见光吸收光谱对Pr-ZnO进行了表征。降解苯酚试验结果表明:超声波催化与紫外光催化具有协同作用。Pr掺杂量为0.1%时,使用0.15 g/L的Pr-ZnO 180 min内降解10 mg/L的苯酚,降解率达到99%。催化剂经过4次重复利用后,苯酚降解率仍超过75%。

关键词: 苯酚, 镨掺杂氧化锌, 声光催化

Abstract:

Pr-doped ZnO was synthesized by a co-precipitation method, which were characterized by X-ray diffraction, scanning electron microscope and ultraviolet-visible light absorption spectrum. The experimental results of phenol degradation showed that ultrasonic catalysis and ultraviolet photocatalysis have a synergistic effect. The degradation efficiency of phenol reached 99% when the doping amount of Pr was 0.1%, the concentration of phenol was 10 mg/L, time was 180 min, and the catalyst dosage was 0.15 g/L. After the catalyst was reused four times, the degradation rate of phenol still exceeded 75%.

Key words: phenol, Pr-doped ZnO, sonophotocatalysis

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