碳材料吸附水中PPCPs的研究进展

doi:10.11894/1005-829x.2015.35(10).006

摘要/Abstract

摘要：

随着药物及个人护理品(PPCPs)的广泛使用,水环境中PPCPs的污染越来越严重.吸附技术对于去除PPCPs表现出一定的优势,其中碳材料对PPCPs的吸附去除被广泛研究.针对碳材料(活性炭和碳纳米管)对水体中PPCPs的吸附机理和研究进展进行了总结和分析,并进一步探讨了碳材料在当前应用中存在的问题及今后的发展方向,以促进相关研究工作的发展.

关键词: 药物及个人护理品, 吸附, 碳材料

Abstract:

With the widespread use of pharmaceutical and personal care products(PPCPs),the water environment pollution caused by PPCPs is more and more serious. Adsorption technology has shown the advantages of PPCPs removal to a certain extent,especially,the PPCPs removal by carbon material adsorption is being widely studied. The mechanism and research progress in PPCPs adsorption on carbon materials,including activated carbons and carbon nanotubes,are summarized and analyzed. Furthermore, the current application problems and the future development direction of carbon materials are discussed,so as to promote the development of relevant research.

Key words: pharmaceutical and personal care products(PPCPs), absorption, carbon materials

中图分类号:

X703.1

刘桂芳, 闫红梅, 高远, 朱丽楠, 徐森. 碳材料吸附水中PPCPs的研究进展[J]. 工业水处理, 2015, 35(10): 6-11.

Liu Guifang, Yan Hongmei, Gao Yuan, Zhu Linan, Xu Sen. Research progress in the PPCPs removal from water by carbon material adsorption[J]. INDUSTRIAL WATER TREATMENT, 2015, 35(10): 6-11.

https://www.iwt.cn/CN/Y2015/V35/I10/6

参考文献

[1] Kinsinger N M,Dudchenko A,Wong A,et al. Synergistic effect of pH and phase in a nanocrystalline titania photocatalyst[J]. Appl. Mater. Interfaces,2013,5(13):6247-6254.
[2] Yang Xin,Flowers R C,Weinberg H S,et al. Occurrence and removal of pharmaceuticals and personal care products(PPCPs) in an advanced wastewater reclamation plant[J]. Water Research,2011,45(16):5218-5228.
[3] 宋存义,汪翠萍,李晖. 污水处理中几种去除药物及个人护理用品方法的机理及效果比较[J]. 环境工程学报,2009,3(11):19211928.
[4] 赵琦,何小娟,唐翀鹏,等. 药物和个人护理用品(PPCPs)处理方法研究进展[J]. 净水技术,2010,29(4):5-10.
[5] Abdelmelek S B,Greaves J,Ishida K P,et al. Removal of pharmaceutical and personal care products from reverse osmosis retentate using advanced oxidation processes[J]. Environ. Sci. Technol.,2011, 45(8):3665-3671.
[6] 乔铁军,张锡辉,欧慧婷. 饮用水中药品和个人护理用品的研究进展[J]. 给水排水,2010,36(4):118-122.
[7] Mestre A S,Pires J,Nogueira J M F,et al. Activated carbons for the adsorption of ibuprofen[J]. Carbon,2007,45:1979-1988.
[8] Yu Zirui,Prldszus S,Huck P M. Adsorption characteristics of selected pharmaceuticals and an endocrine disrupting compound-naproxen,carbamazepine and nonylphenol-on activated carbon[J]. Water Research,2008,429(12):2873-2882.
[9] Ji Liangliang,Liu Fengling,Xu Zhaoyi,et al. Adsorption of pharmaceutical antibiotics on template-synthesized ordered micro-and mesoporous carbons[J]. Environ. Sci. Technol.,2010,44(8):3116-3122.
[10] Liu Hai,Zhang Jian,Bao Nan,et al. Textural properties and surface chemistry of lotus stalk-derived activated carbons prepared using different phosphorus oxyacids:Adsorption of trimethoprim[J]. Journal of Hazardous Materials,2012,235/236:367-375.
[11] Ji Liangliang,Chen Wei,Duan Lin,et al. Mechanisms for strong adsorption of tetracycline to carbon nanotubes:A comparative study using activated carbon and graphite as adsorbents[J]. Environ. Sci. Technol.,2009,43(7):2322-2327.
[12] Zhou Gang,Duan Wenhui,Gu Binglin. First-principles study on morphology and mechanical properties of single-walled carbon nanotube[J]. Chem. Phys. Lett.,2001,333(5):344-349.
[13] Pan Bo,Xing Baoshan. Adsorption mechanisms of organic chemicals on carbon nanotubes[J]. Environ. Sci. Technol.,2008,42(24): 9005-9013.
[14] Helland A,Wick P,Koehler A,et al. Reviewing the environmental and human health knowledge base of carbon nanotubes[J]. Environ. Health Persp.,2007,115:1125-1131.
[15] 王哲,于水利. 碳纳米管对磺胺甲恶唑的吸附过程及其机理研究[J]. 安全与环境学报,2013,13(3):102-105.
[16] Zhang Di,Pan Bo,Zhang Huang,et al. Contribution of different sulfamethoxazole species to their overall adsorption on functionalized carbon nanotubes[J]. Environ. Sci. Technol.,2010,44:3806-3811.
[17] Ji L L,Chen W,Zheng S R,et al. Adsorption of sulfonamide antibiotics to multiwalled carbon nanotubes[J]. Langmuir,2009,25(19):11608-11613.
[18] Hickey J P,Passinoreader D R. Linear solvation energy relationships: Rules of thumb for estimation of variable values[J]. Environ. Sci. Technol.,1991,25:1753-1760.
[19] Nam S W,Choi D J,Kim S K,et al. Adsorption characteristics of selected hydrophilic and hydrophobic micropollutants in water using activated carbon[J]. Journal of Hazardous Materials,2014,270:144-152.
[20] Tappe W,Zarfl C,Kummer S,et al. Growth-inhibitory effects of sulfonamides at different pH:Dissimilar susceptibility patterns of a soil bacterium and a test bacterium used for antibiotic assays[J].Chemosphere,2008,72(5):836-843.
[21] Pyrzynska K,Stafiej A,Biesaga M. Sorption behavior of acidic herbieides on carbon nanotubes[J]. Microchimica Acta,2007,159(3/4):293-298.
[22] Gotovac S,Song L,Kanoh H,et al. Assembly structure control of single wall carbon nanotubes with liquid phase naphthalene adsorption[J]. Colloids and Surfaces A,2007,300(l/2):117-121.
[23] Lu C S,Chung Y L,Chang K F. Adsorption thermodynamic and kinetic studies of trihalomethanes on multiwalled carbon nanotubes[J]. J. Hazard. Mater.,2006,138(2):304-310.
[24] Piao L Y,Liu Q R,Li Y D,et al. Adsorption of L-phenylalanine on single-walled carbon nanotubes[J]. J. Phys. Chem. C,2008,112: 2857-2863.
[25] Cho H H,Smith B A,Wnuk J D,et al. Influence of surface oxides on the adsorption of naphthalene onto multiwalled carbon nanotubes[J]. Environ. Sci. Technol.,2008,42(8):2899-2905.
[26] Liao Qiu,Sun Jing,Gao Lian. The adsorption of resorcinol from water using multi-walled carbon nanotubes[J]. Colloids and Surfaces A:Physicochemical and Engineering Aspects,2008,312(2/3): 160-165.
[27] Choi K J,Kim S G,Kim S H. Removal of tetracycline and sulfonamide classes of antibiotic compound by powdered activated carbon[J]. Environmental Technology,2008,29(3):333-342.
[28] Altmann J,Ruhl A S,Zietzschmann F K,et al. Direct comparison of ozonation and adsorption onto powdered activated carbon for micropollutant removal in advanced wastewater treatment[J]. Water Research,2014,55:185-193.
[29] Nowotny N,Epp B,von Sonntag C,et al. Quantification and modeling of the elimination behavior of ecologically problematic wastewater micropollutants by adsorption on powdered and granulated activated carbon[J]. Environ. Sci. Technol.,2007,41(6):20502055.
[30] Pouretedal H R,Sadegh N. Effective removal of Amoxicillin,Cephalexin,Tetracycline and Penicillin G from aqueous solutions using activated carbon nanoparticles prepared from vine wood[J]. Journal of Water Process Engineering,2014,1:64-73.
[31] Rivera-Utrilla J,Gomez-Pacheco C V,Sanchez-Polo M, et al. Tetracycline removal from water by adsorption/bioadsorption on activated carbons and sludge-derived adsorbents[J]. Journal of Environmental Management,2013,131:16-24.
[32] Sun Yuanyuan,Yue Qinyan,Gao Baoyu,et al. Adsorption and cosorption of ciprofloxacin and Ni(Ⅱ) on activated carbon: Mechanism study[J]. Journal of the Taiwan Institute of Chemical Engineers, 2014,45(2):681-688.
[33] Cho H H,Huang H,Schwab K. Effects of solution chemistry on the adsorption of ibuprofen and triclosan onto carbon nanotubes[J]. Langmuir,2011,27(21):12960-12967.
[34] Peng Hongbo,Pan Bo,Wu Min,et al. Adsorption of ofloxacin and norfloxacin on carbon nanotubes:Hydrophobicityand structure-controlled process[J]. Journal of Hazardous Materials,2012,233/ 234:89-96.
[35] 胡翔, 赵娜, 魏杰. 三氯生在碳纳米管上的吸附[J]. 环境工程学报,2009,3(8):1462-1464.
[36] Wu Di,Pan Bo,Wu Min,et al. Coadsorption of Cu and sulfamethoxazole on hydroxylized and graphitized carbon nanotubes[J]. Science of the Total Environment,2012,427/428:247-252.
[37] Li Haibo,Zhang Di,Han Xiaozeng,et al. Adsorption of antibiotic ciprofloxacin on carbon nanotubes:pH dependence and thermodynamics[J]. Chemosphere,2014,95:150-155.
[38] Pan Bo,Zhang Di,Li Hao,et al. Increased adsorption of sulfamethoxazole on suspended carbon nanotubes by dissolved humic acid[J]. Environ. Sci. Technol.,2013,47(14):7722-7728.

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